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Okay, so the correct answer is both but not simultaneously. Season one, the main character was Crowley. The show opens with Crowly establishing his role in the apocalypse and as a demon who's just not so demon-like. We see him time and time again conversing with different demons, moreso than Aziraphale talks to angels I'm pretty sure. It's Crowley who wants to run away when things go south, and the audience sees this in his "talk" with God. He's the one that freezes time to talk to Adam, he offers his apartment, etc.
Season two our main character is clearly Aziraphale. He's trying to help Jim while doing some soul searching of his own. It's focused more on his understanding of himself and of the Almighty and how he fits into the picture. We follow Aziraphale to Edinburough and even in the flashbacks it's all about his journey to where he is now, back in heaven.
throwing this into the wind and disappearing again. engage in dialogue:
my argument: aziraphale because he’s the one going through the plot defining character arc, and who we’re in the pov of in most of the flashbacks. meanwhile crowley’s the extremely plot relevant close second sexy deuteragonist who’s going through intense mental turmoil and huge stakes like lucy gray. challenge my argument tho